In the past century, superconductivity has been observed in thousands of substances with multifarious chemical compositions and crystal structures; however, researchers have still not found an explicit method for discovering new superconductors. For the unconventional high-Tc superconductors of cuprates and iron pnictides/chalcogenides, the occurrence of superconductivity is highly related to the existence of some certain quasi-two-dimensional structural motifs, e.g., the CuO2 planes or the Fe2As2/Fe2Se2 layers. Thus, low dimensionality has generally been considered as a favorable ingredient for exotic electron pairing due to the enhancement of electronic correlations. While among the quasi-one-dimensional (Q1D) compounds, only a few compounds were found to be superconducting at considerably low temperatures of several degrees Kelvin.